By Norman H. March
In this introductory chemical physics textbook, the authors talk about the interactions, bonding, electron density, and experimental options of loose molecules, and follow spectroscopic the right way to confirm molecular parameters, dynamics, and chemical reactions.
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Additional info for Chemical Physics of Free Molecules
The power of the ESCA technique is clearly in evidence in this direct demonstration of spin splitting of core levels in paramagnetic molecules. 4. Molecular Spectroscopy and Molecular Properties In addition to the techniques already considered in this chapter, other spectroscopic methods are available that yield important information about molecular properties. The atoms in a molecule vibrate around an equilibrium position, and, of course, the molecule as a whole rotates. These modes of motion give rise to various types of spectroscopic results.
Some of these techniques will then be considered in somewhat more detail in later chapters, when they relate directly to predictions made by wave mechanics. *While the atomic masses enter the vibrational frequency and reduce it as the masses are increased, the force constant is a property of the bond itself. CD ... : a:UJ D. c: _rn OlE C:o CD ... 2. Trends in bond properties and predicted bond orders in first-row diatomic molecules [redrawn from Pimentel and Spratley (1969), p. 115]. 8. 1. Background In discussing some of the important experimental methods used in the study of the chemical physics of free molecules, it is useful to start by considering the energy relationships involved when dealing with ionic substances by utilizing the so-called Born-Haber cycle.